Physics, Applied

Article Chemistry, Multidisciplinary

Charge Relays via Dual Carbon-Actions on Nanostructured BiVO4 for High Performance Photoelectrochemical Water Splitting

Yuxiang Wang, Daoming Chen, Jingnan Zhang, M-Sadeeq (Jie Tang) Balogun, Pingshan Wang, Yexiang Tong, Yongchao Huang

Summary: Carbon doping and introduction of carbon quantum dots can improve the electronic conductivity and light absorption capability of BiVO4, thus enhancing the separation and transfer of photo-generated charges. Electroplating a polyaniline layer onto the catalyst can sustain a stable photocurrent density for a long time.

ADVANCED FUNCTIONAL MATERIALS (2022)

Article Chemistry, Multidisciplinary

Achieving 19% Power Conversion Efficiency in Planar-Mixed Heterojunction Organic Solar Cells Using a Pseudosymmetric Electron Acceptor

Wei Gao, Feng Qi, Zhengxing Peng, Francis R. Lin, Kui Jiang, Cheng Zhong, Werner Kaminsky, Zhiqiang Guan, Chun-Sing Lee, Tobin J. Marks, Harald Ade, Alex K-Y Jen

Summary: By adopting the asymmetric selenium substitution strategy and using a pseudosymmetric electron acceptor, the power conversion efficiency of planar-mixed heterojunction organic solar cells (PMHJ OSCs) can be significantly improved. The increased dielectric constant and improved dimer packing lead to lower exciton binding energy, more efficient exciton dissociation, and reduced radiative recombination loss. These findings provide an effective way to develop highly efficient acceptor materials for OSCs.

ADVANCED MATERIALS (2022)

Article Chemistry, Physical

Multifunctional T3C2Tx-(Fe3O4/polyimide composite films with Janus structure for outstanding electromagnetic interference shielding and superior visual thermal management

Yali Zhang, Zhonglei Ma, Kunpeng Ruan, Junwei Gu

Summary: In this study, flexible multifunctional polymer-based electromagnetic interference (EMI) shielding composite films with Janus properties were prepared. The composite films exhibited excellent EMI shielding performance, mechanical properties, and electrothermal and photothermal conversion capabilities.

NANO RESEARCH (2022)

Article Optics

Twin-field quantum key distribution over 830-km fibre

Shuang Wang, Zhen-Qiang Yin, De-Yong He, Wei Chen, Rui-Qiang Wang, Peng Ye, Yao Zhou, Guan-Jie Fan-Yuan, Fang-Xiang Wang, Wei Chen, Yong-Gang Zhu, Pavel Morozov, Alexander Divochiy, Zheng Zhou, Guang-Can Guo, Zheng-Fu Han

Summary: The research team presents an experimental QKD system that can tolerate channel loss and achieve a secure distance of 833.8 km, setting a new record for fibre-based QKD. The optimized protocol and high-quality setup result in a significantly higher secure key rate compared to previous records over similar distances. This breakthrough marks a significant step towards establishing reliable and efficient terrestrial quantum-secure networks over a scale of 1,000 km.

NATURE PHOTONICS (2022)

Review Chemistry, Multidisciplinary

Direct Ink Writing: A 3D Printing Technology for Diverse Materials

M. A. S. R. Saadi, Alianna Maguire, Neethu T. Pottackal, Md Shajedul Hoque Thakur, Maruf Md Ikram, A. John Hart, Pulickel M. Ajayan, Muhammad M. Rahman

Summary: Direct ink writing (DIW) is a versatile 3D printing technique that allows printing of a wide range of materials. This comprehensive review explores the process of DIW printing of complex 3D structures and discusses its diverse applications in various industries.

ADVANCED MATERIALS (2022)

Review Chemistry, Physical

Regulations of active moiety in single atom catalysts for electrochemical hydrogen evolution reaction

Peng Zhu, Xiang Xiong, Dingsheng Wang

Summary: Hydrogen production from water splitting using renewable electric energy is a key topic for achieving a carbon neutral future. Single atom catalysts (SACs) have emerged as a new frontier in catalysis, particularly in the hydrogen evolution reaction (HER), due to their high activity and excellent chemical selectivity. However, the influence of the neighboring coordinated atoms from the supports is often neglected in the classification of SACs. This review proposes a new classification method based on the type of supports and highlights the importance of the metal-support interaction and coordination environment. Structural designing strategies are also proposed to address the current challenges in SACs for HER.

NANO RESEARCH (2022)

Review Chemistry, Multidisciplinary

Prussian Blue Analogues for Sodium-Ion Batteries: Past, Present, and Future

Jian Peng, Wang Zhang, Qiannan Liu, Jiazhao Wang, Shulei Chou, Huakun Liu, Shixue Dou

Summary: This review provides an overview of Prussian blue analogues (PBAs), including material-level optimization and their prospects in practical sodium-ion batteries. It aims to bridge the gap between laboratory research and commercial application.

ADVANCED MATERIALS (2022)

Article Chemistry, Multidisciplinary

Oxygen Vacancy-Induced Dielectric Polarization Prevails in the Electromagnetic Wave-Absorbing Mechanism for Mn-Based MOFs-Derived Composites

Yue Liu, Xinfeng Zhou, Zirui Jia, Hongjing Wu, Guanglei Wu

Summary: Polymeric metal-organic framework (MOF)-derived composites are functional materials with exceptional chemical homogeneity, designable components, and adjustable pore size. This study presents the design of laminate-stacked sphere-shaped trimetallic CoNiMn-MOFs and the successful synthesis of CoNi/MnO@C composites, which exhibit excellent electromagnetic wave-absorbing performance. The modulation of oxygen and Mn vacancies through the introduction of heteroatoms and changes in annealing temperature contributes to the improvement of electromagnetic loss capacity.

ADVANCED FUNCTIONAL MATERIALS (2022)

Review Nanoscience & Nanotechnology

Interfacial Engineering Strategy for High-Performance Zn Metal Anodes

Bin Li, Xiaotan Zhang, Tingling Wang, Zhangxing He, Bingan Lu, Shuquan Liang, Jiang Zhou

Summary: This article reviews the role of interfacial engineering in inhibiting the growth of Zn dendrites and the occurrence of side reactions. Researchers have regulated the deposition behavior of Zn ions through surface modification and the addition of electrolyte additives to achieve uniform Zn nucleation and flat Zn deposition, improving the cycling stability of Zn anodes.

NANO-MICRO LETTERS (2022)

Article Energy & Fuels

Solar cell efficiency tables (Version 61)

Martin A. Green, Ewan D. Dunlop, Gerald Siefer, Masahiro Yoshita, Nikos Kopidakis, Karsten Bothe, Xiaojing Hao

Summary: This article presents consolidated tables that provide an extensive listing of the highest independently confirmed efficiencies for solar cells and modules. It outlines the guidelines for including results into these tables and reviews new entries since July 2022. The article also includes graphs showing the progress of each cell technology over the past 30 years and an updated list of designated test centers.

PROGRESS IN PHOTOVOLTAICS (2023)

Article Chemistry, Multidisciplinary

Hierarchical Engineering of Double-Shelled Nanotubes toward Hetero-Interfaces Induced Polarization and Microscale Magnetic Interaction

Panbo Liu, Yi Wang, Guozheng Zhang, Ying Huang, Ruixuan Zhang, Xianhu Liu, Xuefeng Zhang, Renchao Che

Summary: Hierarchical double-shelled nanotubes (DSNTs) exhibit efficient microwave absorption due to their desirable heterogeneous interfaces, multiple magnetic heteroatomic components, and hollow hierarchical microstructures.

ADVANCED FUNCTIONAL MATERIALS (2022)

Review Chemistry, Multidisciplinary

Critical Review on Low-Temperature Li-Ion/Metal Batteries

Nan Zhang, Tao Deng, Shuoqing Zhang, Changhong Wang, Lixin Chen, Chunsheng Wang, Xiulin Fan

Summary: This article presents a comprehensive research on the key factors contributing to the poor low-temperature performance of LIBs and proposes strategies and solutions to improve it.

ADVANCED MATERIALS (2022)

Article Nanoscience & Nanotechnology

Biomass-Derived Carbon Heterostructures Enable Environmentally Adaptive Wideband Electromagnetic Wave Absorbers

Zhichao Lou, Qiuyi Wang, Ufuoma Kara, Rajdeep S. Mamtani, Xiaodi Zhou, Huiyang Bian, Zhihong Yang, Yanjun Li, Hualiang Lv, Solomon Adera, Xiaoguang Wang

Summary: This study presents the design of carbon heterostructures derived from bamboo, which exhibit excellent electromagnetic absorption performance and environmental adaptability. The assembly of nanofibers and nanosheets acts as a nanometer-sized antenna, enhancing the conductive loss. The composition of cellulose and lignin in the precursor significantly affects the assembly shape, the formation of covalent bonds, and the surface hydrophobicity. The obtained carbon heterostructure maintains wideband electromagnetic absorption in real-world environments.

NANO-MICRO LETTERS (2022)

Review Chemistry, Multidisciplinary

Chemodynamic Therapy via Fenton and Fenton-Like Nanomaterials: Strategies and Recent Advances

Chenyang Jia, Yuxin Guo, Fu-Gen Wu

Summary: Chemodynamic therapy (CDT) is a novel cancer treatment strategy that generates hydroxyl radicals in the tumor region using Fenton or Fenton-like reactions. It has advantages such as low side effects, independence from external stimulation, modulation of the tumor microenvironment, and low treatment cost. CDT can also be combined with other therapies to enhance anticancer effects.
Review Chemistry, Multidisciplinary

Surface Passivation Using 2D Perovskites toward Efficient and Stable Perovskite Solar Cells

Guangbao Wu, Rui Liang, Mingzheng Ge, Guoxing Sun, Yuan Zhang, Guichuan Xing

Summary: 3D perovskite solar cells face challenges in surface defects and material interplay. 2D perovskites provide better stability as a protective barrier. Surface passivation using 2D perovskites enables higher efficiency and stability.

ADVANCED MATERIALS (2022)

Article Nanoscience & Nanotechnology

High-Efficiency Electromagnetic Interference Shielding of rGO@FeNi/Epoxy Composites with Regular Honeycomb Structures

Ping Song, Zhonglei Ma, Hua Qiu, Yifan Ru, Junwei Gu

Summary: With the rapid development of fifth-generation mobile communication technology and wearable electronic devices, the need for highly efficient EMI shielding materials has become crucial. In this study, a three-dimensional graphene oxide (GO) with regular honeycomb structure (GH) was constructed using sacrificial template and freeze-drying methods. Amino functionalized FeNi alloy particles (f-FeNi) were loaded onto the GH skeleton followed by in-situ reduction to prepare rGH@FeNi aerogel. The resulting rGH@FeNi/epoxy composites with a low rGH@FeNi mass fraction of 2.1 wt% exhibited a high EMI shielding effectiveness (EMI SE) of 46 dB, which is 5.8 times higher than that of rGO/FeNi/epoxy composites with the same mass fraction. The composites also displayed excellent thermal stability and mechanical properties.

NANO-MICRO LETTERS (2022)

Review Chemistry, Physical

Insight on Organic Molecules in Aqueous Zn-Ion Batteries with an Emphasis on the Zn Anode Regulation

Donghong Wang, Qing Li, Yuwei Zhao, Hu Hong, Hongfei Li, Zhaodong Huang, Guojin Liang, Qi Yang, Chunyi Zhi

Summary: This study assesses the basic reactions and progress on the anode side of rechargeable aqueous zinc ion batteries (AZIBs), investigates the role of organic molecules in stabilizing the zinc anode, and proposes strategies for further exploration of high performance batteries.

ADVANCED ENERGY MATERIALS (2022)

Article Chemistry, Multidisciplinary

Initiating VB-Group Laminated NbS2 Electromagnetic Wave Absorber toward Superior Absorption Bandwidth as Large as 6.48 GHz through Phase Engineering Modulation

Huibin Zhang, Junye Cheng, Honghan Wang, Zehao Huang, Qingbin Zheng, Guangping Zheng, Deqing Zhang, Renchao Che, Maosheng Cao

Summary: VB-Group NbS2 nanosheets prepared through a facile one-step solvothermal method exhibit remarkable electromagnetic wave absorption performance, showing tunable absorbing frequency bands (C-, X-, and Ku-bands) and the ability to adjust performance by changing material contents.

ADVANCED FUNCTIONAL MATERIALS (2022)

Article Chemistry, Multidisciplinary

Record-Efficiency Flexible Perovskite Solar Cells Enabled by Multifunctional Organic Ions Interface Passivation

Lu Yang, Jiangshan Feng, Zhike Liu, Yuwei Duan, Sheng Zhan, Shaomin Yang, Kun He, Yong Li, Yawei Zhou, Ningyi Yuan, Jianning Ding, Shengzhong (Frank) Liu

Summary: A novel compound HADI was designed to improve the efficiency and stability of flexible perovskite solar cells, showing significant roles in surface modification, passivation, and charge transfer. PSCs based on HADI-SnO2 electron transport layer exhibited outstanding performance.

ADVANCED MATERIALS (2022)

Article Chemistry, Multidisciplinary

Quenching-Resistant Multiresonance TADF Emitter Realizes 40% External Quantum Efficiency in Narrowband Electroluminescence at High Doping Level

Pengcheng Jiang, Jingsheng Miao, Xiaosong Cao, Han Xia, Ke Pan, Tao Hua, Xialei Lv, Zhongyan Huang, Yang Zou, Chuluo Yang

Summary: This study introduces a highly emissive molecule with enhanced quenching resistance by segregating the planar MR-TADF skeleton using two bulky carbazolyl units, which significantly improves the performance of corresponding devices with a maximum external quantum efficiency of 40.0% and a full width at half maximum of 25 nm. The steric effect of the bulky carbazolyl units largely removes the formation of detrimental excimers/aggregates, leading to an OLED example that can achieve narrow bandwidth and high EL efficiency surpassing 40% to date.

ADVANCED MATERIALS (2022)