期刊
GREEN CHEMISTRY
卷 16, 期 7, 页码 3528-3538出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4gc00004h
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资金
- Alexander von Humboldt Foundation
- Federal Ministry of Education and Research
- Max Planck Society
- ERC Advanced Grant
- German federal and state governments to promote science and research at German universities
Recently, the mechanocatalytic depolymerization of lignocelluloses yielding 'water-soluble lignocelluloses' was demonstrated. Water-soluble C-5 & C-6 sugars and sulfur-free lignins are formed through the saccharification of the oligosaccharides, allowing for the fractionation of biomass by simple filtration. Herein, we present an in-depth analysis of water-soluble products obtained from beechwood. The complex nature of the 'water-soluble beechwood' is investigated by 2D HSQC NMR, HPLC and gel filtration chromatography. The detailed analysis of the `water-soluble beechwood' lends significant insights into the chemical nature of the lignocellulose depolymerization driven by the mechanical forces.
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