期刊
GREEN CHEMISTRY
卷 13, 期 10, 页码 2759-2763出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c1gc15434f
关键词
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资金
- Deutsche Forschungsgemeinschaft (DFG)
- Graduate School of Molecular Science
A new and straightforward method to transform carbohydrate-based biomass to formic acid (FA) by oxidation with molecular oxygen in aqueous solution using a Keggin-type H(5)PV(2)Mo(10)O(40) polyoxometalate as catalyst is presented. Several water-soluble carbohydrates were fully and selectively converted to formic acid and CO(2) under very mild conditions. It is worth noting, even complex biomass mixtures, such as poplar wood sawdust, were transformed to formic acid, giving 19 wt% yield (11% based on the carbon atoms in the feedstock) under non-optimized conditions.
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