期刊
GREEN CHEMISTRY
卷 12, 期 8, 页码 1376-1379出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c0gc00136h
关键词
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资金
- National Science Foundation [CHE 05-43133]
- Robert A. Welch Foundation [A-0923]
- CAPES (Brazil)
The coupling of oxetane (trimethylene oxide) and carbon dioxide catalyzed by VO(acac)(2), in the presence of an onium salt was studied. The process was found to be highly selective and quantitative for the production of the six-membered cyclic carbonate, trimethylene carbonate, under very mild reaction conditions of 60 degrees C and 1.7 MPa. Other derivatives of trimethylene oxide were shown to similarly selectively afford the corresponding cyclic carbonates upon reaction with CO(2).
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