期刊
GEOPHYSICAL RESEARCH LETTERS
卷 37, 期 -, 页码 -出版社
AMER GEOPHYSICAL UNION
DOI: 10.1029/2010GL044951
关键词
-
资金
- Office of Naval Research [N00014-10-1-0811]
- NASA
- NRC
- NOAA [NA06OAR4310082]
- ONR [N00014-04-1-0118]
- NSF [ATM-0340832]
Airborne measurements in regions of varying meteorology and pollution are used to quantify the contribution of organic acids and a mass spectral marker for oxygenated aerosols, m/z 44, to the total organic aerosol budget. Organic acids and m/z 44 separately are shown to exhibit their highest organic mass fractions in the vicinity of clouds. The contribution of such oxygenated species is shown to increase as a function of relative humidity, aerosol hygroscopicity (and decreasing organic mass fraction), and is typically greater off the California coast versus the continental atmospheres studied. Reasons include more efficient chemistry and partitioning of organic acid precursors with increasing water in the reaction medium, and high aqueous-phase processing times in boundary layers with higher cloud volume fractions. These results highlight the importance of secondary organic aerosol formation in both wet aerosols and cloud droplets. Citation: Sorooshian, A., S. M. Murphy, S. Hersey, R. Bahreini, H. Jonsson, R. C. Flagan, and J. H. Seinfeld (2010), Constraining the contribution of organic acids and AMS m/z 44 to the organic aerosol budget: On the importance of meteorology, aerosol hygroscopicity, and region, Geophys. Res. Lett., 37, L21807, doi: 10.1029/2010GL044951.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据