4.2 Article

Multi-colour pulses from seeded free-electron-lasers: towards the development of non-linear core-level coherent spectroscopies

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FARADAY DISCUSSIONS
卷 171, 期 -, 页码 487-503

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ROYAL SOC CHEMISTRY
DOI: 10.1039/c4fd00100a

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资金

  1. European Research Council [202804-TIMER]
  2. Italian Ministry of University and Research [FIRB-RBAP045JF2, FIRB-RBAP06AWK3]
  3. Regional Government of Friuli Venezia Giulia [Nanotox 0060-2009]

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We report on new opportunities for ultrafast science thanks to the use of two-colour extreme ultraviolet (XUV) pulses at the FERMI free electron laser (FEL) facility. The two pulses have been employed to carry out a pioneering FEL-pump/FEL-probe diffraction experiment using a Ti target and tuning the FEL pulses to the M-2/3-edge in order to explore the dependence of the dielectric constant on the excitation fluence. The future impact that the use of such a two-colour FEL emission will have on the development of ultrafast wave-mixing methods in the XUV/soft X-ray range is addressed and discussed.

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