期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 137, 期 33, 页码 10472-10475出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b05960
关键词
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资金
- National Basic Research Program [2013CB834502]
- National Natural Science Foundation of China [91027006, 21125417, 21434005]
- Key Science Technology Innovation Team of Zhejiang Province [2013TD02]
- Open Project of State Key Laboratory of Supramolecular Structure and Materials [sklssm201509]
Here we developed a novel CO2-responsive pillararene-based molecular recognition motif established from a water-soluble pillar[5]arene and an anionic surfactant, sodium dodecyl sulfonate (SDS). The inclusion complex acted as a supramolecular amphiphile and self-assembled into spherical bilayer vesicles as confirmed by DLS, SEM, and TEM experiments. These vesicles were disrupted upon bubbling N-2 or adding much more SDS to eliminate the inclusion complex. The assembly and disassembly of vesicles were successfully employed in gas and surfactant triggered releases of calcein, a water-soluble dye.
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