期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 137, 期 49, 页码 15410-15413出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b11129
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资金
- School of Physical Sciences at the University of California, Irvine
- Chao Family Comprehensive Cancer Center
A synthetic approach to paxilline indole diterpenes is described. The route to the pentacydic core relies on a new regioselective alkenylation of ketones and a tandem radical addition-aldol reaction sequence to access vicinal quaternary stereocenters. Emindole SB, the simplest member of the family, is synthesized in 11 steps from commercially available material to demonstrate the application of this approach.
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