期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 137, 期 46, 页码 14586-14589出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b10267
关键词
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资金
- MOST [2015CB856600]
- NSFC [21332001, 21431008]
- Peking-Tsinghua Center for Life Sciences
- China Postdoctoral Science Foundation [2014 M550546]
Selective cleavage of an inert C-C bond followed by C-O/N bond formation through a long-distance aryl migration from a carbon to a nitrogen center via Ag catalysis is reported. The migration products were easily converted into gamma-hydroxy amines and tetrahydroquinoline derivatives in quantitative yields. Preliminary mechanistic studies indicated a radical pathway.
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