期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 138, 期 1, 页码 108-111出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b12263
关键词
-
资金
- National Science Foundation [CHE-1004924]
The first total synthesis of (+/-)-gelsenicine is reported. The synthetic route is highly efficient (13 steps), featuring (1) a pivotal metal-catalyzed isomerization/rearrangement process that forges the central core of the molecule and (2) two facile C-N bond-forming steps that establish the flanking heterocycles.
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