期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 137, 期 7, 页码 2460-2463出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja5130012
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资金
- ERATO program from JST
- JSPS [26888007]
- World Premier International Research Center (WPI) Initiative, Japan
- Grants-in-Aid for Scientific Research [26888007] Funding Source: KAKEN
Versatile imidation of aromatic C-H bonds was accomplished. In the presence of copper bromide and 6,6'-dimethyl-2,2'-bipyridyl, a range of aromatics, such as polycyclic aromatic hydrocarbons, aromatic bowls, porphyrins, heteroaromatics, and natural products, can be imidated by N-fluorobenzenesulfonimide. A dramatic ligand-accelerated copper catalysis and an interesting kinetic profile were uncovered.
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