期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 137, 期 37, 页码 11868-11871出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b06828
关键词
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资金
- European Research Council [ERC AdG 247014]
- Swedish Research Council [621-2013-4653]
- Berzelii Center EXSELENT
- Knut and Alice Wallenberg Foundation
A highly efficient palladium-catalyzed oxidative cascade reaction of enallenes undergoing overall four C-C bond formations has been developed. The insertion cascade proceeds via carbonylation carbocyclization carbonylation alkynylation involving sequential insertion of carbon monoxide, olefin, and carbon monoxide. Furthermore, different types of terminal alkynes and functionalized enallenes have been investigated and found to undergo the cascade reaction under mild reaction conditions.
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