期刊
JOURNAL OF SOLID STATE CHEMISTRY
卷 224, 期 -, 页码 45-51出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jssc.2014.03.030
关键词
Carbon nanotube; Reduced graphene oxide; Nanohybrid; Supercapacitor
资金
- Ministry of Education, Singapore [MOE2011-T2-2-062, 2013-T1-002-132]
- Asian Office of Aerospace Research and Development of the U.S. Air Force Research Laboratory [FA23861314110]
We report the synthesis of a free-standing two dimensional carbon nanotube (CNT)-reduced graphene oxide (rGO) hybrid by directly growing CNTs on air-sprayed GO paper. As a result of the good integration between CNTs and thermally reduced GO film during chemical vapor deposition, excellent electrical conductivity (2.6 x 10(4) S/m), mechanical flexibility (electrical resistance only increases 1.1% after bent to 90 for 500 times) and a relatively large surface area (3353 m(2)/g) are achieved. Two-electrode supercapacitor assembled using the CNT-rGO hybrids in ionic liquid electrolyte (1-ethyl-3-methylimidazolium tetrafluoroborate) shows excellent stability upon 500 bending cycles with the gravimetric energy density measuring 23.7 Wh/kg and a power density of 2.0 kW/kg. Furthermore, it shows an impedance phase angle of -64.4 degrees at a frequency of 120 Hz, suggesting good potentials for 120 Hz alternating current line filtering applications. (C) 2014 Elsevier Inc. All rights reserved.
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