4.8 Article

Increase in NOx Emissions from Indian Thermal Power Plants during 1996-2010: Unit-Based Inventories and Multisatellite Observations

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ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷 46, 期 14, 页码 7463-7470

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AMER CHEMICAL SOC
DOI: 10.1021/es300831w

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  1. National Aeronautics and Space Administration (NASA)
  2. Office of Biological and Environmental Research in the U.S. Department of Energy, Office of Science
  3. U.S. Department of Energy [DE-AC02-06CH11357]

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Driven by rapid economic development and growing electricity demand, NOx emissions (E) from the power sector in India have increased dramatically since the mid 1990s In this study, we present the NOx emissions from Indian public thermal power plants for the period 1996-2010 using a unit-based methodology and compare the emission estimates with the satellite observations of NO2 tropospheric vertical column densities (TVCDs) from four space-borne instruments: GOME, SCIAMACHY, OMI, and GOME-2. Results show that NO emissions from Indian power plants increased by at least 70% during 1996-2010. Coal-fired power plants, NOx emissions from which are not regulated in India, contribute similar to 96% to the total power sector emissions, followed by gas-fired (similar to 4%) and oilfired (<1%) ones. A number of isolated NO2 hot spots are observed over the power plant areas, and good agreement between NO2 TVCDs and NOx emissions is found for areas dominated by power plant emissions. Average NO2 TVCDs over power plant areas were continuously increasing during the study period. We find that the ratio of Delta E/E to Delta TVCD/TVCD changed from greater than one to less than one around 2005-2008, implying that a transition of the overall NOx chemistry occurred over the power plant areas, which may cause significant impact on the atmospheric environment.

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