期刊
ENVIRONMENTAL EARTH SCIENCES
卷 70, 期 5, 页码 2387-2395出版社
SPRINGER
DOI: 10.1007/s12665-013-2530-9
关键词
Sorption; Cesium and iodide; Distribution coefficient (K-d); Sorption-affecting factors; Bentonite buffer; Radioactive waste repository
资金
- National Research Foundation of Korea (NRF)
- Korean government (MEST)
The sorption of cesium and iodide ions onto KENTEX-bentonite was investigated using batch test and in-diffusion test methods. The cesium ions were highly sorbed on the bentonite, and the experimental data fit the Freundlich isotherm well. The distribution coefficient, K (d), of the cesium ions was variably affected by the chemical conditions of the solution (initial ion concentration, pH, salinity) and temperature. An increasing pH of solution increased the K (d). However, there were different K (d) values that decrease with an increase in the initial ion concentration, salinity, and temperature. The iodide ions, on the contrary, were negligibly sorptive. The K (d) values obtained from the in-diffusion tests were quite lower than those from the batch tests, which could be explained by changes in the pore water chemistry and surface area available for sorption.
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