Lead isotopes in environmental sciences:: A review

Lead (Pb) isotopic analyses proved to be a very efficient tool for tracing the sources of local and global Pb pollution. This review presents an overview of literature published on the use of Pb isotopic analyses of different environmental matrices (atmospheric aerosols, lichens, tree rings, peat deposits, lake, stream, marine sediments, soils, etc.). In order to gain more insight, the isotopic compositions of major sources of Pb in the environment as determined by several authors are described in detail. These include, above all, the former use of leaded gasoline, coal combustion, industrial activities (e.g., metallurgy) and waste incineration. Furthermore, this review summarises analytical techniques (especially ICP-MS) used for the determination of Pb isotopes in environmental samples. (C) 2007 Elsevier Ltd. All rights reserved.