期刊
JOURNAL OF POWER SOURCES
卷 293, 期 -, 页码 562-569出版社
ELSEVIER
DOI: 10.1016/j.jpowsour.2015.05.092
关键词
Lithium ion battery; LiTi2(PO4)(3); Aqueous electrolyte; Carbon coating; High rate; Good cycling life
资金
- Fok Ying Tung Foundation [NRC07/08.EG01]
- Science and Information Technology of Guangzhou Municipal [2014J4500002, 2014J4500025]
In this study, a one-pot sintering process incorporating sol gel preparation route and in-situ carbon coating was proposed for the synthesis of carbon-coated nanosized LiTi2(PO4)(3). Experimental results show that the prepared LiTi2(PO4)(3) particles are of high crystallinity and well-coated by turbostratic carbon. Attributed to nanosized particles and enhanced conductivity provided by turbostratic carbon coating, the carbon-coated LiTi2(PO4)(3) showed high rate performance and good cycling life in aqueous electrolyte. Particularly, the carbon-coated LiTi2(PO4)(3) exhibited initial specific capacities of 103 and 89 mAh g(-1), and retained 80.6% and 97% of the initial capacities after 120 cycles at 1C and 10C in aqueous electrolyte, respectively. The high rate performance and good cycling life of carbon-coated LiTi2(PO4)(3) in aqueous electrolyte reveal its potential as negative electrode in aqueous lithium-ion batteries for electric vehicles and industrial-scale energy storage systems. (C) 2015 Elsevier B.V. All rights reserved.
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