期刊
ENERGY SOURCES PART A-RECOVERY UTILIZATION AND ENVIRONMENTAL EFFECTS
卷 33, 期 8, 页码 785-794出版社
TAYLOR & FRANCIS INC
DOI: 10.1080/15567030903261899
关键词
hydrogen; jet fuel; kinetic model; reaction mechanisms; reformation; supercritical water
资金
- U.S. Army through DRS Technical Services, Inc. [0602705]
An experimental kinetic study was performed on the supercritical water reformation of jet fuel to account for the interactive contributions of three principal reactions that are taking place, viz., non-catalytic reformation of original and fragmented hydrocarbon molecules, pyrolysis of hydrocarbon molecules, and water gas shift reaction. Experiments were conducted non-catalytically using supercritical water and jet fuel in a specially designed 926 mL Inconel 625 Grade-1 tubular reactor at temperatures varying from 803 to 972 K at a pressure of 24.15 +/- 0.06 MPa. The Arrhenius activation energies and frequency factors were obtained for each of the three principal reactions.
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