期刊
JOURNAL OF POWER SOURCES
卷 273, 期 -, 页码 1098-1102出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2014.07.067
关键词
Lithium-ion battery; Dynamic electrochemical impedance spectroscopy; Single frequency impedance; Charge and discharge differences
资金
- National Natural Science Foundation of China [51207080]
- Independent Research Programs of Tsinghua University [2011Z01004]
- China Postdoctoral Science Foundation [2012M510436]
In this study, a novel implementation of dynamic electrochemical impedance spectroscopy (DEIS) is proposed. The method first measures the impedance continuously at a single frequency during one charging/discharging cycle, then repeats the measurement at a number of other selected frequencies. The impedance spectrum at a specific SOC is obtained by interpolating and collecting the impedance at all of the selected frequencies. The charge transfer resistance, R-ct, from the DEIS is smaller than that from the steady EIS in a wide state-of-charge (SOC) range from 0.4 to 1.0, the R-ct during charging is generally smaller than that during discharging for the battery chemistry used in this study. (C) 2014 Published by Elsevier B.V.
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