4.7 Article

Mechanistic Insights into Thermal Stability Improvement of exo-Tetrahydrodicyclopentadiene by a New Hydrogen Donor: 5,6,7,8-Tetrafluoro-1,2,3,4-tetrahydroquinoxaline

期刊

ENERGY & FUELS
卷 29, 期 1, 页码 16-20

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AMER CHEMICAL SOC
DOI: 10.1021/ef5016445

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资金

  1. Korea University
  2. Korea Institute of Energy Technology Evaluation and Planning (KETEP) Human Resources Development [2011-4010203050]
  3. National Research Foundation of Korea (NRF) Nuclear Research and Development Program

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We investigated the thermal stability of exo-tetrahydrodicyclopentadiene (exo-THDCP, C10H16) in the absence and presence of 5,6,7,8-tetrafluoro-1,2,3,4-tetrahydroquinoxaline (TFQox), a new hydrogen donor (H donor). Conversion of exo-THDCP was slowed in the presence of TFQox but less effectively compared to its analogues, 1,2,3,4-tetrahydroquinoxaline (THQox) and 1,2,3,4-tetrahydroquinoline (THQ). We analyzed the H-donor effects on the thermal decomposition kinetics of exo-THDCP, which explains the relative effect of the H donors on the thermal stability improvement of exo-THDCP.

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