期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 7, 期 1, 页码 297-301出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ee43214a
关键词
-
资金
- Office of Science of the U.S. Department of Energy [DE-SC0004993]
The development of practical solar-driven electrochemical fuel generators requires the integration of light absorbing and electrochemical components into an architecture that must also provide easy separation of the product fuels. Unfortunately, many of these components are not stable under the extreme pH conditions necessary to facilitate ionic transport between redox reaction sites. By using a controlled recirculating stream across reaction sites, this work demonstrates a stable, self-regulating and continuous purified solar-hydrogen generation from near neutral pH electrolytes that yield continuous nearly pure H-2 streams with solar-fuel efficiencies above 6.2%.
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