期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 5, 期 6, 页码 7323-7327出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ee21653a
关键词
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资金
- Natural Science Foundation of China [51107076]
- Education Department of China [210125]
- China Postdoctoral Science Foundation [20110491570]
- Outstanding Young Scientist Foundation of Shandong Province [BS2009NJ014]
- Key Sci-Tech Development Project of Shandong Province [2009GG10007006]
- Shandong University of Technology
Here we show that the introduction of N into a carbon surface facilitates the hydrogen-bonding interactions between the carbon surface and CO2 molecules, which accounts for the superior CO2 uptake of the N-doped activated carbons. This new finding challenges the long-held viewpoint that acid-base interactions between N-containing basic functional groups and acidic CO2 gas are responsible for the enhanced CO2 capture capacity of N-doped carbons.
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