4.8 Article

Photocatalytic H2 production in aqueous solution with host-guest inclusions formed by insertion of an FeFe-hydrogenase mimic and an organic dye into cyclodextrins

期刊

ENERGY & ENVIRONMENTAL SCIENCE
卷 5, 期 8, 页码 8220-8224

出版社

ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ee22109h

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资金

  1. Natural Science Foundation of China [20633020, 21120102036]
  2. Basic Research Program of China [2009CB220009]
  3. Swedish Energy Agency
  4. Swedish Research Council
  5. K & A Wallenberg Foundation

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Bio-inspired noble-metal-free supramolecular systems were constructed by host-guest inclusions of an FeFe-hydrogenase mimic and an organic dye into cyclodextrins respectively, which give typically a ninefold increase in the TON, a sixteenfold enhancement in the quantum efficiency, and a threefold extension in lifetime as compared to the same system in the absence of cyclodextrin for photocatalytic H-2 production in aqueous solution.

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