期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 2, 期 4, 页码 397-400出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b814539c
关键词
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资金
- Specially Promoted Research [19350077]
- Ministry of Education, Culture, Sports, Science and Technology of Japan
We have detected the first example of open porous metal-organic frameworks (MOFs) that functions as an activity site for the reduction of water into hydrogen molecules in the presence of Ru(bpy)(3)(2+), MV2+, and EDTA-2Na under visible light irradiation. This activity is highly efficient: the turnover number based on MOFs and the apparent quantum yield are 8.16 and 4.82%, respectively. Furthermore, this material enables the adsorption of various gases into its pores; its hydrogen uptake capacity is 1.2 wt% at 77.4 K.
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