期刊
ELECTROCHIMICA ACTA
卷 123, 期 -, 页码 340-345出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2013.12.156
关键词
Vapor grown carbon fiber; Carbon black; Polymer actuator; Large strain; Electrochemical
资金
- KAKENHI from the Japan Society for the Promotion of Science (JSPS) [24550264]
- Grants-in-Aid for Scientific Research [24550264] Funding Source: KAKEN
The electrochemical and electromechanical properties of poly(vinylidene fluoride-co-hexafluoropropylene) based actuators using carbon black (CB)/vapor grown carbon fiber (VGCF)/ionic liquid (IL) composite gel electrodes formed without ultrasonication were compared with those of actuators using only CB or VGCF. The double-layer capacitance of the CB/VGCF/IL electrodes was larger than that of the CB/IL electrodes and increased with VGCF content. The amount of strain exhibited by the CB/VGCF/IL actuators was also larger than that for the CB/IL actuators, with the highest strain being produced for an actuator with a CB:VGCF ratio of 1:1. This was slightly larger than that for a polymer actuator using single-walled carbon nanotubes (SWCNTs), indicating that the proposed actuators exhibit sufficiently high performance for real-world applications without the need for expensive SWCNTs. Furthermore, the frequency dependence of the displacement response of the CB/VGCF/IL polymer actuators was successfully simulated using an electrochemical kinetic model similar to that for SWCNT-based actuators. The results yielded the strain in the low-frequency limit and the time constant of the response. (C) 2014 Elsevier Ltd. All rights reserved.
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