期刊
ELECTROCHIMICA ACTA
卷 85, 期 -, 页码 162-168出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2012.08.040
关键词
Molybdenum sulfide; Graphene flake; Counter electrode; Electrocatalytic activity; Dye-sensitized solar cell
资金
- National Science Council in Taiwan [NSC-101-2221-E-036-035]
- National High Technology Research and Development Program of China [2009AA03Z217]
- National Natural Science Foundation of China [90922028, 50842027]
In this study, a composite film of molybdenum sulfide (MoS2)/graphene flake was characterized as the counter electrode (CE) for Pt-free dye-sensitized solar cells (DSSCs). It was found that the enhanced electrocatalytic activity can be demonstrated when high-conductive graphene flake was introduced into MoS2 film. The cyclic voltammograms showed that the cathodic current density of MoS2/graphene CE was higher than those of MoS2, graphene and Pt CEs due to its lamellar structure. Additionally, MoS2/graphene CE exhibited a low charge-transfer resistance of 2.17 Omega cm(2). After the optimization in the thickness of MoS2/graphene CE, the power conversion efficiency of the DSSC assembled with the optimized MoS2/graphene reached 5.98% under AM1.5 illumination of 100 mW cm(-2), which is comparable to that based on the Pt CE. (C) 2012 Elsevier Ltd. All rights reserved.
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