4.2 Article

Wave-packet propagation based calculation of above-threshold ionization in the x-ray regime

出版社

IOP PUBLISHING LTD
DOI: 10.1088/0953-4075/48/12/124001

关键词

free-electron lasers; ab initio calculations; x-ray photoionization; above-threshold ionization

资金

  1. DAAD RISE program
  2. Deutsche Forschungsgemeinschaft [SFB 925]

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We investigate the multi-photon process of above-threshold ionization for the light elements hydrogen, carbon, nitrogen, and oxygen in the hard x-ray regime. Numerical challenges are discussed and by comparing Hartree-Fock-Slater calculations with configuration-interaction-singles results we justify the mean-field potential approach in this regime. We present a theoretical prediction of two-photon above-threshold-ionization cross sections for the mentioned elements. Moreover, we study how the importance of above-threshold ionization varies with intensity. We find that for carbon, at x-ray intensities around 1023 W cm(-2), two-photon above-threshold ionization of the K-shell electrons is as probable as one-photon ionization of the L-shell electrons.

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