期刊
ELECTROCHEMISTRY COMMUNICATIONS
卷 40, 期 -, 页码 45-48出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.elecom.2013.12.022
关键词
Lithium-oxygen battery; Composite protective layer; Lithium metal anode; Electrolyte; Cycling stability
资金
- National Research Foundation of Korea (NRF)
- Korean government (MEST) [NRF-2009-0094219]
Lithium-oxygen batteries are of great interest because of their very high-energy density; however, they present many challenges, one of which is the low-cycling stability of a lithium (Li) metal anode. Here, we report a composite protective layer (CPL) comprising Al2O3 and polyvinylidene fluoride-hexafluoro propylene for a Li metal anode that resulted in a dramatic enhancement of the cycling stability of a lithium-oxygen battery. A cell with the CPL-coated Li metal anode exhibited more than 3 times higher discharge capacity at the 80th cycle compared to a cell without the CPL X-ray photoelectron spectroscopy measurements for the cycled lithium metal anodes confirm that the CPL effectively suppressed electrolyte decomposition at the surface of the Li metal anode. Published by Elsevier B.V.
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