期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 6, 期 12, 页码 2367-2378出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.5b00716
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资金
- Australian Research Council of ARC Future Fellowships
- Australian Government through Australian Renewable Energy Agency (ARENA)
Molecular materials afford abundant flexibility in the tunability of physical and electronic properties. As such, they are ideally suited to engineering low-cost, flexible, light-harvesting materials that break away from the single-threshold paradigm. Single-threshold solar cells are capable of harvesting a maximum of 33.7% of incident sunlight, whereas two-threshold cells are capable of energy harvesting efficiencies exceeding 45%. In this Perspective, we provide the theoretical background with which upper efficiency limits for various multiple-threshold solar cell architectures may be calculated and review and discuss various reports that employ processes such as triplet triplet annihilation and singlet fission in multiple-threshold devices comprised of molecular materials.
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