期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 120, 期 1, 页码 771-780出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.5b11094
关键词
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资金
- Korea Research Fellowship Program through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT and Future Planning [2015H1D3A1066333]
- Universiti Kebangsaan Malaysia (UKM) [GUP-2014-012]
- Ministry of Higher Education Malaysia [FRGS/1/2013/SG02/UKM/01/1]
- National Research Foundation of Korea [2015H1D3A1066333] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
A simple low-temperature solution processed bismuth-doped ZnO nanorods (NRs) and poly(3-hexylthiophene) (P3HT) were used as electron acceptor and donor, respectively, in a hybrid inorganic-organic photovoltaic system. Controlling Bi precursor concentration via solution processing (hydrothermal method) plays an important role in altering the morphology, structure, and intrinsic defects of ZnO NRs. Interstitial doping of BiBi2O3 into ZnO (BiZO) NRs results in simultaneous improvement of the open circuit voltage and short circuit current density primarily due to prolonged charge carrier recombination lifetime, increased donor-acceptor interfacial areas with efficient exciton dissociation, and charge carrier mobility. As a result, the power conversion efficiency of the 2 wt % BiZO NRs-P3HT device was significantly enhanced by 55% compared with that of the pristine device. Overall, our study highlighted the immense potential of BiZO NRs as an excellent electron acceptor for fabrication of hybrid optoelectronic devices.
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