Isotopic constraints on intensified aridity in Central Asia around 12 Ma

The relationship between central Asian acidification and the evolution of the Himalayan-Tibetan orogen remains elusive. New isotopic data from pedogenic and lacustrine carbonates sampled from well-dated Neogene strata (15.7-1.8 Ma) in the northeastern Qaidam basin of the northern Tibetan Plateau identify a positive shift of similar to 2.5 parts per thousand in delta O-18 values from 12 Ma to 10.7 Ma. High values were maintained until similar to 3.3 Ma when delta O-18 values drop by 1 parts per thousand. The timing of the positive shift in delta O-18 values is remarkably consistent with isotopic records from a vast region along and within the northern Tibetan Plateau. Isotopic, mineralogical, petrologic, and facies analyses suggest that diagenetic effects and detrital contamination are minimal. The positive shift in delta O-18 values, as well as high delta C-13 values from pedogenic carbonates (which are suggestive of low soil respiration rates), is interpreted to indicate intensified aridity in central Asia ca. 12 Ma. The recognition of intensified aridity is critical to understanding the climatic effects of the development of the Himalayan-Tibetan orogen. We attribute this climatic change in the central Asia to: (1) retreat of Paratethys from central Asia, strengthening the seasonal contrast and resulting in the loss of a nearby moisture source; (2) attainment of high elevations in the Himalayas and south-central Tibet, blocking moisture-bearing air masses from the Indian and Pacific oceans; and (3) enhanced isolation and outward growth of the northern Tibetan Plateau. The negative shift around 3.3 Ma might be related to the onset of Northern Hemisphere glaciation, intensification of the East Asia monsoon, and/or effects of orographic rain-out. (C) 2011 Elsevier B.V. All rights reserved.