4.6 Article

Facile synthesis of nanoporpous graphitic carbon nitride photocatalyst coupled with N-doped graphene quantum dots for efficient photo degradation dyes under nature solar light radiation

期刊

DIAMOND AND RELATED MATERIALS
卷 89, 期 -, 页码 197-205

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.diamond.2018.09.012

关键词

Metal-free photocatalyst; In-situ synthesis; Nanoporous; Photocatalytic degradation

资金

  1. National Natural Science Foundation of China [51773184]
  2. Shanxi Provincial Natural Science Foundation of China [201701D121046]

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Nanoporous graphitic carbon nitride modified with N-doped graphene quantums dots (N-GQD@npg-C3N4) was prepared via a one-pot co-sintering method. The presented N-GQD@npg-C3N4 showed a high photocatalytic activity (PCA) for the degradation of organic dyes under solar radiation. This result can be ascribed to two reasons: (i) the uniform distribution of N-GQDs on the surface of npg-C3N4, which allows for an accelerated electron transfer from npg-C3N4 to N-GQD; and (ii) the unique nanoporous structure of npg-C3N4, providing a large active surface area. This work opens up a new avenue for the utilization of a robust, cost-effective and metal-free photocatalyst in practical applications, e.g. waste water treatment.

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