期刊
DALTON TRANSACTIONS
卷 -, 期 44, 页码 9708-9711出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/b913823d
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资金
- Ministry of Education, Culture, Sports, Science and Technology, Japan [19020061]
- Kansai Research Foundation for Technology Promotion (KRF)
- Japan Society for the Promotion of Science (JSPS) for Young Scientists
Vanadium(IV) complexes bearing 3-hydroxypicolinic acid (H(2)hpic) as ligands, VO(Hhpic)(2) (1) and the cyclic tetramer (VO)(4)(hpic)(4) (2), have excellent catalytic ability for the oxidation of a variety of primary and secondary benzyl alcohols with molecular oxygen in acetonitrile or protic solvents such as ethanol and water, affording the corresponding aldehydes and ketones, respectively. Construction of multi-nuclear complexes by the selection of ligands attains higher turnover numbers and recycling of the catalyst.
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