期刊
CRYSTAL GROWTH & DESIGN
卷 13, 期 8, 页码 3528-3534出版社
AMER CHEMICAL SOC
DOI: 10.1021/cg400500t
关键词
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资金
- Chemical Sciences, Geo-sciences, and Biosciences Division, Office of Basic Energy Sciences, U.S. Department of Energy [DEFG02-03ER15457, DE-FG02-99ER14999]
- Department of Defense through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program
- ANSER Center, an Energy Frontier Research Center
- U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-SC0001059]
Through a combination of protecting groups, postsynthesis deprotection, and postsynthesis metallation, a homogeneously inaccessible, single-site vanadyl-(monocatecholate) moiety can be incorporated into the dipyridyl struts of a Zn-based, pillared paddlewheel MOF. The resulting MOF, which has large pores, exhibits catalytic activity in the benzylic oxidation of tetralin in the presence of tert-butylhydroperoxide.
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