期刊
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
卷 343, 期 1-3, 页码 34-42出版社
ELSEVIER
DOI: 10.1016/j.colsurfa.2009.01.026
关键词
Polyion; Electrostatic repulsions; Polyelectrolyte-decorated particles
Interaction of charged particles, induced by adding an oppositely charged polyion, gives rise to intriguing aggregation phenomena. The presence of short-range interactions in competition with electrostatic repulsions results, in an interval of concentrations around the inversion point, in the formations of long-lived clusters of polyelectrolyte-decorated particles. We will show that the whole aggregation scenario can be justified as due to an heterogeneous charge distribution at the particle surface, as a consequence of the correlated polyion adsorption, on the basis of a recently model proposed by D. Velegol, R Thwar, Langmuir 17 (2001) 7687-7693. (C) 2009 Elsevier B.V. All rights reserved.
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