期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 54, 期 31, 页码 9057-9060出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201502194
关键词
dehydrogenation; homogeneous catalysis; hydrogen; iridium; methanol
资金
- KAKENHI [25105732, 26620153, 26288047]
- Asahi Glass Foundation
- Grants-in-Aid for Scientific Research [26288047, 26620153, 25105732] Funding Source: KAKEN
An efficient catalytic system for the production of hydrogen from a methanol-water solution has been developed using a new anionic iridium complex bearing a functional bipyridonate ligand as a catalyst. This system can be operated under mild conditions [weakly basic solution (0.046molL(-1) NaOH) below 100 degrees C] without the use of an additional organic solvent. Long-term continuous hydrogen production from a methanol-water solution catalyzed by the anionic iridium complex was also achieved.
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