期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 54, 期 27, 页码 7939-7943出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201502206
关键词
biomass; graphitic carbon; heterogeneous catalysis; hydrogenation; stability
资金
- Center for Biorenewable Chemicals (CBiRC) - NSF [EEC-0813570]
- NSF [DGE-1256259]
Conversion of biomass-derived molecules involves catalytic reactions under harsh conditions in the liquid phase (e.g., temperatures of 250 degrees C and possibly under either acidic or basic conditions). Conventional oxide-supported catalysts undergo pore structure collapse and surface area reduction leading to deactivation under these conditions. Here we demonstrate an approach to deposit graphitic carbon to protect the oxide surface. The heterogeneous catalysts supported on the graphitic carbon/oxide composite exhibit excellent stability (even under acidic conditions) for biomass conversion reactions.
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