期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 55, 期 5, 页码 1868-1871出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201509888
关键词
asymmetric catalysis; cyclizations; heterocycles; hydrogen bonds; organocatalysis
资金
- HKUST
- Hong Kong RGC [GRF 604513, ECS605812, M-HKUST607/12]
A new asymmetric synthesis of chiral 1,4-dioxanes and other oxa-heterocycles has been developed by means of organocatalytic enantioselective desymmetrization of oxetanes. This mild process proceeds with exceedingly high efficiency and enantioselectivity to establish the quaternary stereocenters. This method complements the existing, yet limited, strategies for the synthesis of these oxa-heterocycles.
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