期刊
CHEMSUSCHEM
卷 7, 期 4, 页码 1051-1056出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201301218
关键词
biofuels; electrochemistry; energy conversion; heterogeneous catalysis; oxidation reaction
资金
- Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences
This study demonstrates that an electrochemical dehydrogenation process can be used to oxidize glycerol to glyceraldehyde and glyceric acid even without using stoichiometric chemical oxidants. A glyceric acid selectivity of 87.0% at 91.8% glycerol conversion was obtained in an electrocatalytic batch reactor. A continuous-flow electrocatalytic reactor had over an 80% high glyceric acid selectivity at 10% glycerol conversion, as well as greater reaction rates than either an electrocatalytic or a conventional catalytic batch reactor.
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