期刊
CHEMSUSCHEM
卷 7, 期 11, 页码 2998-3001出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201402311
关键词
alcohols; biomass; carboxylic acids; hydrogenation; ruthenium
资金
- KRICT [KK-1401-B0]
Catalytic hydrogenation of organic carboxylic acids and their esters, for example, cellulosic ethanol from fermentation of acetic acid and hydrogenation of ethyl acetate is a promising possibility for future biorefinery concepts. A hybrid conversion process based on selective hydrogenation of butyric acid combined with fermentation of glucose has been developed for producing biobutanol. ZnO-supported Ru-Sn bimetallic catalysts exhibits unprecedentedly superior performance in the vapor-phase hydrogenation of biomass-derived butyric acid to n-butanol (>98% yield) for 3500h without deactivation.
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