期刊
CHEMSUSCHEM
卷 7, 期 2, 页码 442-450出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201301140
关键词
density functional calculations; dye/pigments; electrochemistry; energy conversion; hafnium
资金
- 863 Program [2009AA03Z220]
- NSFC [50773008]
- National Science&Technology Pillar Program [2012BAD47B02]
- Shaanxi Provincial Department of Education [2010JK655, 2013JK0927]
- Sci-Tech R&D Program of Shaanxi Province [2010K01-120, 2011JM6010]
- SRF for ROCS, SEM
Mesoporous-graphitic-carbon-supported HfO2 (HfO2-MGC) nanohybrids were synthesized by using a soft-template route. Characterization and a systematic investigation of the catalytic properties, stability, and catalytic mechanism were performed for HfO2-MGC counter electrodes (CEs) in dye-sensitized solar cells (DSSCs). The new HfO2-MGC as a CE in DSSCs showed a surprisingly high efficiency of 7.75% for the triiodide/iodide redox couple and 3.69% for the disulfide/thiolate redox couple, greater than the Pt electrode in the corresponding electrolyte system, which opens up a possibility for its practical application.
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