期刊
CHEMPHYSCHEM
卷 14, 期 1, 页码 125-131出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cphc.201200734
关键词
cavity; J-aggregates; polariton; strong coupling; time-resolved spectroscopy
资金
- ERC [227577]
- icFRC (International Center for Frontier Research in Chemistry)
- European Research Council (ERC) [227577] Funding Source: European Research Council (ERC)
We present a comprehensive experimental study of the photophysical properties of a moleculecavity system under strong coupling conditions, using steady-state and femtosecond time-resolved emission and absorption techniques to selectively excite the lower and upper polaritons as well as the reservoir of uncoupled molecules. Our results demonstrate the complex decay routes in such hybrid systems and that, contrary to expectations, the lower polariton is intrinsically long-lived.
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