期刊
CHEMPHYSCHEM
卷 10, 期 4, 页码 680-685出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cphc.200800672
关键词
core/shell structures; luminescence; nanoparticles; quantum dots; surfactants
资金
- National Natural Science Foundation of China [20501005, 20771037]
- Program for New Century Excellent Talents in University of China [NCET-06-0417]
- Pujiang Talents Project [07pj14032]
- Shuguang Project [06SG33]
- SRFDP [20070251014]
An effective shell-coating route is developed for covering oil-soluble CdTe quantum dots (QDs), which usually tend to aggregate during the heating-up process involved in shell formation. The new route is based on balancing the coordinating capacity and the activation effect of selected surfactants. The thus obtained highly luminescent CdTe/CdS core/shell QDs exhibit photoluminescence quantum yields as high as 92%-among the best results obtained so far for luminescent semiconductor nanocrystals. By changing the size of the CdTe core, or the thickness of the CdS shell, the emission colors of the obtained core/shell nanocrystals can be tuned between the visible and near-infrared regions of the spectrum following an identical procedure.
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