期刊
CHEMOMETRICS AND INTELLIGENT LABORATORY SYSTEMS
卷 139, 期 -, 页码 156-167出版社
ELSEVIER
DOI: 10.1016/j.chemolab.2014.09.014
关键词
Baseline correction; Baseline drift; Sparse derivative; Asymmetric penalty; Low-pass filtering; Convex optimization
类别
资金
- NSF [CCF-1018020]
- Direct For Computer & Info Scie & Enginr
- Division of Computing and Communication Foundations [1018020] Funding Source: National Science Foundation
This paper jointly addresses the problems of chromatogram baseline correction and noise reduction. The proposed approach is based on modeling the series of chromatogram peaks as sparse with sparse derivatives, and on modeling the baseline as a low-pass signal. A convex optimization problem is formulated so as to encapsulate these non-parametric models. To account for the positivity of chromatogram peaks, an asymmetric penalty function is utilized. A robust, computationally efficient, iterative algorithm is developed that is guaranteed to converge to the unique optimal solution. The approach, termed Baseline Estimation and Denoising With Sparsity (BEADS), is evaluated and compared with two state-of-the-art methods using both simulated and real chromatogram data. (C) 2014 Elsevier B.V. All rights reserved.
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