期刊
CHEMISTRY-AN ASIAN JOURNAL
卷 7, 期 4, 页码 642-657出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.201100772
关键词
hydrogen; oxygen; photocatalysis; solar energy; water splitting
资金
- Scientific Research Foundation of East China University of Science and Technology [YD0142125]
- Science and Technology Commission of Shanghai Municipality [09J1402800, 10JC1403200]
- Education Commission of Shanghai Municipality [09SG27]
- National Natural Science Foundation of China [20973059, 91022023, 21076076]
- Fundamental Research Funds for the Central Universities [WJ0913001]
- Programme for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning
- Programme for New Century Excellent Talents in University [NCET-09-0347]
Photocatalytic water splitting using semiconductor photocatalysts has been considered as a green process for converting solar energy into hydrogen. The pioneering work on electrochemical photolysis of water at TiO2 electrode, reported by Fujishima and Honda in 1972, ushered in the area of solar fuel. As the real ultimate solution for solar fuel-generation, overall water splitting has attracted interest from researchers for some time, and a variety of inorganic photocatalysts have been developed to meet the challenge of this dream reaction. To date, high-efficiency hydrogen production from pure water without the assistance of sacrificial reagents remains an open challenge. In this Focus Review, we aim to provide a whole picture of overall water splitting and give an outlook for future research.
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