期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 20, 期 21, 页码 6264-6267出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201400332
关键词
carbon dioxide; heterogeneous catalysis; hydrogenation; methylation; platinum
资金
- JSPS [25106010]
- MEXT
- Grants-in-Aid for Scientific Research [26289299, 25106010] Funding Source: KAKEN
Pt and MoOx co-loaded TiO2 is found to be highly effective for direct methylation of aliphatic and aromatic secondary amines by CO2 and H-2 under solvent-free conditions. This is the first additive-free and reusable heterogeneous catalytic system with acceptable turnover number.
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