期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 20, 期 11, 页码 2990-2996出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201304376
关键词
carbon dioxide; frustrated Lewis pairs; main group elements; organocatalysis; reduction
资金
- National Sciences and Engineering Research Council of Canada (NSERC, Canada)
- Centre de Catalyse et Chimie Verte (Quebec)
- NSERC
- FQRNT
Metal-free systems, including frustrated Lewis pairs (FLPs) have been shown to bind CO2. By reducing the Lewis acidity and basicity of the ambiphilic system, it is possible to generate active catalysts for the deoxygenative hydroboration of carbon dioxide to methanol derivatives with conversion rates comparable to those of transition-metal-based catalysts.
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