期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 20, 期 33, 页码 10220-10222出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201403321
关键词
amine functionalization; CO2 capture; photocatalysis; solar fuels; TiO2
资金
- NTU
- MOE AcRF [RG 44/11, MOE2012-T2-2-041, ARC 5/13]
- CRP from NRF Singapore [NRF-CRP5-2009-04]
Amine-functionalization of TiO2 nanoparticles, through a solvothermal approach, substantially increases the affinity of CO2 on TiO2 surfaces through chemisorption. This chemisorption allows for more effective activation of CO2 and charge transfer from excited TiO2, and significantly enhances the photocatalytic rate of CO2 reduction into methane and CO.
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