期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 20, 期 51, 页码 16853-16857出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201404565
关键词
alkyl azaarenes; iminium catalysis; Michael addition; palladium; synergistic catalysis
资金
- European Regional Development Fund (ERDF) through the INTERREG IV A France (Channel)-England cross-border cooperation programme [4061]
- Engineering and Physical Sciences Research Council [EP/K029150/1] Funding Source: researchfish
- EPSRC [EP/K029150/1] Funding Source: UKRI
A novel catalytic enantioselective methodology based on synergistic catalysis is reported. The strategy involves: 1) the metal-Lewis-acid activation of alkylazaarenes, and 2) the secondary-amine activation of enals. Consequently, highly functionalized chiral alkylazaarenes were obtained in good yields and with reasonable stereoselectivity.
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