期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 19, 期 32, 页码 10589-10594出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201300899
关键词
aldehydes; carbonylation; hydroformylation; phosphine; ruthenium
资金
- Bundesministerium fur Bildung und Forschung (the German Federal Ministry of Education and Research) [03X3559]
- Swiss National Science Foundation
- Chinese Scholarship Council
The ruthenium-catalyzed hydroformylation of 1- and 2-octene to give preferentially the corresponding linear aldehyde is reported. The catalyst system comprising of Ru-3(CO)(12) and an imidazole-substituted monophosphine ligand allows for high chemo-and regioselectivity. The hydroformylation proceeds with unprecedented rates for a ruthenium-based catalyst.
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